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Title

Time-resolved monitoring of polycyclic aromatic hydrocarbons adsorbed on atmospheric particles
Authors
Subtil Sousa, Gustavo Alexandre
Kiselev, Denis
Kasparian, Jérôme
George, Christian
Ferreira, José
Favreau, Philippe
Lazzarotto, Benoît
Wolf, Jean-Pierre
Published in Environmental science and pollution research international. 2017, vol. 24, no. 24, p. 19517-19523
Abstract Real-time monitoring of individual particles from atmospheric aerosols was performed by means of a specifically developed single-particle fluorescence spectrometer (SPFS). The observed fluorescence was assigned to particles bearing polycyclic aromatic hydrocarbons (PAH). This assignment was supported by an intercomparison with classical speciation on filters followed by gas chromatography-mass spectrometry (GC-MS) analysis. As compared with daily-averaged data, our time resolved approach provided information about the physicochemical dynamics of the particles. In particular, distinctions were made between background emissions related to heating, and traffic peaks during rush hours. Also, the evolution of the peak fluorescence wavelength provided an indication of the aging of the particles during the day.
Keywords Aerosols — Monitoring — Fluorescence — Polycyclic aromatic hydrocarbons — Identification — Pollution — Real time
Identifiers
arXiv: 1707.05177
Note arXiv: 1707.05177 - http://arxiv.org/abs/1707.05177
Full text
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Article (Published version) (1.2 MB) - document accessible for UNIGE members only Limited access to UNIGE
Other version: http://link.springer.com/10.1007/s11356-017-9612-2
Structures
Centres et instituts / Institut des sciences de l'environnement
Faculté des sciences / Section de physique / Groupe de physique appliquée
Research groups ISE Climat
ISE Pôle Sciences
Projects
Swiss National Science Foundation: NCCR MUST
European Commission: LIPBA
Citation
(ISO format) 		SUBTIL SOUSA, Gustavo Alexandre et al. Time-resolved monitoring of polycyclic aromatic hydrocarbons adsorbed on atmospheric particles. In: Environmental science and pollution research international, 2017, vol. 24, n° 24, p. 19517-19523. doi: 10.1007/s11356-017-9612-2 https://archive-ouverte.unige.ch/unige:95493

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Deposited on : 2017-07-19

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