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Title

Modelling of HNO3-mediated laser-induced condensation: A parametric study

Authors
Rohwetter, P.
Wöste, L.
Published in Journal of Chemical Physics. 2011, vol. 135, no. 13, p. 134703
Abstract Based on both static (extended Köhler) and dynamic modelling, we investigate the influence of temperature,humidity, HNO3 initial concentration, as well as of the particle concentration, on the efficiency of HNO3-mediated laser-induced condensation. This mechanism is most efficient for low temperatures, high HNO3 concentration, and relative humidities. It is, however, still active up to 30 °C, down to 70% relative humidity, and below the ppm level of HNO3. Furthermore, lower particle concentration minimizing the depletion of both HNO3 and water vapor is more favourable to particle growth
Keywords Water vaporCondensationAtmospheric waterSolution thermodynamicsVapor pressure
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ISE Climat
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ROHWETTER, P. et al. Modelling of HNO3-mediated laser-induced condensation: A parametric study. In: Journal of Chemical Physics, 2011, vol. 135, n° 13, p. 134703. https://archive-ouverte.unige.ch/unige:37105

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Deposited on : 2014-06-03

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