Doctoral thesis
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Ultrafast Dynamics of Molecular Systems Probed with Time-Resolved Soft X-Ray Absorption Spectroscopy Using Liquid Flat-Jets

ContributorsChang, Yi-Pingorcid
Imprimatur date2023-01-24
Abstract

My thesis relates to the investigation of the ultrafast molecular dynamics involved in the photophysics/ photochemistry of different chemical systems in the gas, mesoscopic and liquid phases, with the element, site, and orbital specificity offered by time-resolved X-ray absorption spectroscopy, which is achieved with a table-top HHG source covering the water window that is combined with liquid flatjet delivery systems capable of delivering submicron thin sheets of liquid samples. These studies are made with the main goal of achieving a better understanding of the effect of the solvent or liquid environment on condensed systems. To that end, different molecular dynamics on the femto- to picosecond timescales have been successfully observed between the gaseous and condensed phases of different systems.

Keywords
  • Liquid flatjet
  • HHG
  • X-ray absorption spectroscopy
  • Ultrafast
Research groups
Citation (ISO format)
CHANG, Yi-Ping. Ultrafast Dynamics of Molecular Systems Probed with Time-Resolved Soft X-Ray Absorption Spectroscopy Using Liquid Flat-Jets. Doctoral Thesis, 2023. doi: 10.13097/archive-ouverte/unige:167789
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Technical informations

Creation03/27/2023 8:41:09 AM
First validation03/28/2023 11:23:16 AM
Update time05/10/2023 11:17:41 AM
Status update05/10/2023 11:17:41 AM
Last indexation11/01/2024 4:37:09 AM
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