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Poor electronic screening in lightly doped Mott insulators observed with scanning tunneling microscopy |
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Published in | Physical review. B, Condensed matter and materials physics. 2017, vol. 95, no. 23 | |
Abstract | The effective Mott gap measured by scanning tunneling microscopy (STM) in the lightly doped Mott insulator (Sr1−xLax)2IrO4 differs greatly from values reported by photoemission and optical experiments. Here we show that this is a consequence of the poor electronic screening of the tip-induced electric field in this material. Such effects are well known from STM experiments on semiconductors and go under the name of tip-induced band bending (TIBB). We show that this phenomenon also exists in the lightly doped Mott insulator (Sr1−xLax)2IrO4 and that, at doping concentrations of x≤4%, it causes the measured energy gap in the sample density of states to be bigger than the one measured with other techniques. We develop a model able to retrieve the intrinsic energy gap leading to a value which is in rough agreement with other experiments, bridging the apparent contradiction. At doping x≈5% we further observe circular features in the conductance layers that point to the emergence of a significant density of free carriers in this doping range and to the presence of a small concentration of donor atoms. We illustrate the importance of considering the presence of TIBB when doing STM experiments on correlated-electron systems and discuss the similarities and differences between STM measurements on semiconductors and lightly doped Mott insulators. | |
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Research group | Groupe Baumberger | |
Citation (ISO format) | BATTISTI, I. et al. Poor electronic screening in lightly doped Mott insulators observed with scanning tunneling microscopy. In: Physical Review. B, Condensed Matter, 2017, vol. 95, n° 23. doi: 10.1103/PhysRevB.95.235141 https://archive-ouverte.unige.ch/unige:101916 |